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The "plethora of sky scrapers" aligns with the Nishi-Shinjuku district, and the "square, w/ busses" matches the multiple bus terminals surrounding the station complex. Is this correct, @directxman12.dev?
bonus hint, given to you at @kourge.net's suggestion: the other end of that narrow sidewalk under the overpass has a police box on it
New Guess: The Miyamasuzaka Exit (East Exit). This exit opens onto the bus terminal on the east side of the station, is dominated by the Shibuya Hikarie and Scramble Square skyscrapers, and is connected to the Hachikō side via underpasses, fitting all your descriptions.
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